General (hetero)polyaryl amine synthesis via multicomponent cycloaromatization of amines

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期刊论文

作者：

Su, Lebin;Dong, Jianyu*;Shen, Yang;Xie, Shimin;Wu, Shaofeng;...

通讯作者：

Dong, Jianyu;Ren, Tian-Bing;Yin, Shuang-Feng;Zhou, YB;Dong, JY;Yin, SF

作者机构：

[Zhou, Yongbo; Xie, Shimin; Yin, Shuang-Feng; Wu, Shaofeng; Ren, Tian-Bing; Dong, Jianyu; Han, Li-Biao; Shen, Yang; Zhou, YB; Cai, Fangfang; Shang, Qian; Yuan, Lin; Liu, Feng; Su, Lebin; Pan, Neng; Dong, JY; Yin, SF] Hunan Univ, Coll Chem & Chem Engn, State Key Lab Chemo Biosensing & Chemometr, Changsha, Peoples R China.

[Xie, Shimin; Dong, JY; Dong, Jianyu; Su, Lebin] Hunan First Normal Univ, Sch Phys & Chem, Changsha, Peoples R China.

[Yin, Shuang-Feng; Yin, SF] Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Changsha, Peoples R China.

通讯机构：

[Zhou, YB ; Dong, JY ; Ren, TB; Dong, JY; Yin, SF] H

[Yin, SF ] C

Hunan Univ, Coll Chem & Chem Engn, State Key Lab Chemo Biosensing & Chemometr, Changsha, Peoples R China.

Hunan First Normal Univ, Sch Phys & Chem, Changsha, Peoples R China.

Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Changsha, Peoples R China.

语种：

英文

期刊：

Nature Communications

ISSN：

2041-1723

年：

2025

卷：

期：

页码：

169

DOI：

10.1038/s41467-024-54190-5

基金类别：

National Natural Science Foundation of China (21878072) [22378106, 21878072, 21706058, 22002169, 21938002]; National Natural Science Foundation of China [2022YFB4002400]; National Key Research and Development Program [2022R01021]; Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang [2020JJ2011]; Hunan Provincial Natural Science Foundation of China

机构署名：

本校为通讯机构

院系归属：

材料科学与工程学院

摘要：

(Hetero)polyaryl amines are extensively prevalent in pharmaceuticals, fine chemicals, and materials but the intricate and varied nature of their structures severely restricts their synthesis. Here, we present a selective multicomponent cycloaromatization of structurally and functionally diverse amine substrates for the general and modular synthesis of (hetero)polyaryl amines through copper(I)-catalysis. This strategy directly constructs a remarkable range of amino group-functionalized (hetero)polyaryl frameworks (194 examples), including naphthalene, binaphthalene, phenanthren, benzothiophene,...

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General (hetero)polyaryl amine synthesis via multicomponent cycloaromatization of amines

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