Cellulose nanofibrils (CNFs), disintegrated from natural fibers, are promising alternatives in wastewater purification for the porous structure and numerous hydroxyls. The pristine CNFs aerogel has limited mechanical strength and are vulnerable to collapse when exposed to water. In this work, eco-friendly and recycled CNFs aerogel adsorbents were successfully prepared using cellulose nanofibrils (CNFs), which cross-linked by poly(vinyl alcohol) (PVA) and acrylic acid (AA). The combination of PVA and AA endowed CNFs aerogel strong three-dimensional porous structure and desirable adsorption prop...