Investigation into the effect of solvents on lignin hydrogenation for the production of phenolic compounds

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成果类型：

期刊论文

作者：

Liu, Chao;Wu, Yiqiang;Cai, Tingting;Chen, Yuwei;Jia, Shuya;...

通讯作者：

Wu, YQ;Jiang, Jianchun;Wang, K

作者机构：

[Li, Zhaoshuang; Liu, Chao; Wu, Zhiping; Qing, Yan; Wu, Yiqiang] Cent South Univ Forestry & Technol, Sch Mat Sci & Engn, Changsha 410004, Peoples R China.

[Jiang, Jianchun; Liu, Chao; Cai, Tingting; Wang, Kui; Wang, K; Jiang, JC] Inst Chem Ind Forest Prod, Chinese Acad Forestry, Key Lab Biomass Energy & Mat Jiangsu Prov, Natl Engn Lab Biomass Chem Utilizat, Nanjing 210042, Jiangsu, Peoples R China.

[Chen, Yuwei] Yancheng Inst Technol, Sch Automot Engn, Yancheng 224051, Peoples R China.

[Zhang, Xiaolei; Jia, Shuya] Univ Strathclyde, Dept Chem & Proc Engn, Glasgow City G1 1XJ, Scotland.

通讯机构：

[Wu, YQ ] C

[Wang, K ; Jiang, JC] I

Cent South Univ Forestry & Technol, Sch Mat Sci & Engn, Changsha 410004, Peoples R China.

Inst Chem Ind Forest Prod, Chinese Acad Forestry, Key Lab Biomass Energy & Mat Jiangsu Prov, Natl Engn Lab Biomass Chem Utilizat, Nanjing 210042, Jiangsu, Peoples R China.

语种：

英文

期刊：

Green Chemistry

ISSN：

1463-9262

年：

2024

卷：

期：

页码：

3356-3367

DOI：

10.1039/d3gc04902g

基金类别：

National Basic Research Program of China (973 Program) [2022YFB4201904]; National Key Research and Development Program of China [32222058]; National Natural Science Foundation; ARCHIE-WeSt, at the University of Strathclyde

机构署名：

本校为第一且通讯机构

院系归属：

材料科学与工程学院

摘要：

Solvents play a critical role in the lignin hydrogenation process. However, elucidating the role of solvents in lignin hydrogenation solely through experimental methods presents considerable challenges. The present report integrates experimental results, quantum chemical calculations, and molecular dynamics simulations to study the effect of solvents on the hydrogenation of lignin on Ru/C to produce phenolic compounds. Solvents not only disperse the substrate and promote the mass transfer process in the hydrogenation reaction, but also signific...

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Investigation into the effect of solvents on lignin hydrogenation for the production of phenolic compounds

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