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Cr-Doped FeNi–P Nanoparticles Encapsulated into N-Doped Carbon Nanotube as a Robust Bifunctional Catalyst for Efficient Overall Water Splitting

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成果类型:
期刊论文
作者:
Wu, Yiqiang;Tao, Xu;Qing, Yan*;Xu, Han;Yang, Fan;...
通讯作者:
Qing, Yan;Lu, Xihong
作者机构:
[Tao, Xu; Wu, Yiqiang; Xu, Han; Liu, Ming; Tian, Cuihua; Luo, Sha; Qing, Yan] Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Hunan Prov Collaborat Innovat Ctr High Efficiency, Changsha 410004, Hunan, Peoples R China.
[Yang, Fan; Lu, Xihong] Sun Yat Sen Univ, Sch Chem, Key Lab Low Carbon Chem & Energy Conservat Guangd, MOE,Key Lab Bioinorgan & Synthet Chem, Guangzhou 510275, Guangdong, Peoples R China.
通讯机构:
[Qing, Yan] C
[Lu, Xihong] S
Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Hunan Prov Collaborat Innovat Ctr High Efficiency, Changsha 410004, Hunan, Peoples R China.
Sun Yat Sen Univ, Sch Chem, Key Lab Low Carbon Chem & Energy Conservat Guangd, MOE,Key Lab Bioinorgan & Synthet Chem, Guangzhou 510275, Guangdong, Peoples R China.
语种:
英文
关键词:
bifunctional catalyst;Cr doping;structural manipulation;transition metals phosphide;water splitting
期刊:
Advanced Materials
ISSN:
0935-9648
年:
2019
卷:
31
期:
15
页码:
e1900178
基金类别:
This work was financially supported by the National Science Foundation of China (31530009, 31500476, 31890771, 31870552, and U1810110), the Young Elite Scientists Sponsorship Program by CAST (2016QNRC001), the Outstanding Innovative Youth Training Program of Changsha (KQ1707019), and the Hunan Provincial Technical Innovation Platform and Talent Program in Science and Technology (2018RS3092, 2018WK4028, and 2016TP1013).
机构署名:
本校为第一且通讯机构
院系归属:
材料科学与工程学院
摘要:
Exploring high-efficiency, stable, and cost-effective bifunctional electrocatalysts for overall water splitting is greatly desirable and challenging. Herein, a newly designed hybrid catalyst with Cr-doped FeNi–P nanoparticles encapsulated into N-doped carbon nanotubes (Cr-doped FeNi–P/NCN) with unprecedented electrocatalytic activity is developed by a simple one-step heating treatment. The as-synthesized Cr-doped FeNi–P/NCN with moderate Cr doping exhibits admirable oxygen evolution reaction and hydrogen evolution reaction activities with ov...

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