Coupling effects between metal-organic framework derivatives and oxygen-deficient TiO2 nanotubes: identified charge-transfer processes and photoelectric synergistic effect

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成果类型：

期刊论文

作者：

Zhang, Honglin;Jia, Meiying;Tong, Jing;Peng, Haihao;Xiang, Yinping;...

通讯作者：

Xiong, WP

作者机构：

[Yang, Zhaohui; Tong, Jing; Xiong, WP; Zhang, Honglin; Peng, Haihao; Xiang, Yinping; Xiong, Weiping] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

[Jia, Meiying] Cent South Univ Forestry & Technol, Coll Environm Sci & Engn, Changsha 410004, Peoples R China.

[Xiong, WP; Chen, Zhaomeng; Xiong, Weiping] Hunan Boke Environm Engn Co Ltd, Hengyang 421099, Peoples R China.

[Xu, Zhengyong] Hunan Modern Environm Technol Co Ltd, Changsha 410004, Peoples R China.

通讯机构：

[Xiong, WP ] H

Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

Hunan Boke Environm Engn Co Ltd, Hengyang 421099, Peoples R China.

语种：

英文

期刊：

Environmental Science: Nano

ISSN：

2051-8153

年：

2023

卷：

期：

页码：

1993-2009

DOI：

10.1039/d3en00223c

基金类别：

The study was financially supported by the National Youth Foundation of China (52000064), the National Natural Science Foundation of China (U20A20323), the Natural Science Foundation of Hunan Province (2023JJ0013), Special Funding for the Construction of Hunan's Innovative Province (2021SK2040) and the Science and Technology Innovation Program of Hunan Province (2021RC3133).

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院系归属：

环境科学与工程学院

摘要：

The in situ self-assembling of metal-organic frameworks (MOFs) to construct thin-film electrodes is a major challenge in designing efficient photoelectric catalysts. In this study, we propose a method for preparing MOF derivative and TiO2 nanotube (TNT) coupled catalysts with S-scheme Ar-ZrO2/Ti2O3-TNTs, where Ar-ZrO2 derived from NH2-UiO-66 was modified in situ inside Ti2O3-TNTs. The TiO2 nanotubes not only played an important role in substrate loading and support but also served as the source of Ti3+ for the self-modifying. Such a photoelectr...

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Coupling effects between metal-organic framework derivatives and oxygen-deficient TiO2 nanotubes: identified charge-transfer processes and photoelectric synergistic effect

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