Universal pseudo-fluctuation engineering induces local free radical surface confinement effect to enhance photocatalytic oxidation of toluene

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成果类型：

期刊论文

作者：

Yuhui Liu;Zhe Wang;Peng Chen;Lang Chen;Shuang-Feng Yin

通讯作者：

Peng Chen<&wdkj&>Lang Chen

作者机构：

[Yuhui Liu; Zhe Wang; Peng Chen] School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, Guizhou 550025, PR China

College of Chemistry and Chemical Engineering, Central South University of Forestry and Technology, Changsha 410004, PR China

[Lang Chen] Advanced Catalytic Engineering Research Center of the Ministry of Education, State Key Laboratory of Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, PR China

[Shuang-Feng Yin] College of Chemistry and Chemical Engineering, Central South University of Forestry and Technology, Changsha 410004, PR China<&wdkj&>Advanced Catalytic Engineering Research Center of the Ministry of Education, State Key Laboratory of Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, PR China

通讯机构：

[Peng Chen] S

[Lang Chen] A

Advanced Catalytic Engineering Research Center of the Ministry of Education, State Key Laboratory of Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Hunan University, Changsha 410082, PR China<&wdkj&>School of Chemistry and Chemical Engineering, Guizhou University, Guiyang, Guizhou 550025, PR China

语种：

英文

关键词：

C−H activation;Photocatalytic toluene oxidation;Long-term selectivity;Free radical;Dynamic regulation

期刊：

Applied Catalysis B: Environmental

ISSN：

0926-3373

年：

2026

卷：

380

页码：

125806

DOI：

10.1016/j.apcatb.2025.125806

机构署名：

本校为其他机构

摘要：

Breaking the trade-off between activity and selectivity has always been a long-standing challenge in the field of catalysis. In this study, we introduce an innovative universal pseudo-fluctuation strategy utilizing surface-uncoordinated In(OH) 3-x -ZnIn 2 S 4 heterojunctions (ZIO) to achieve local free radical confinement. Notably, the low-coordination and contraction of In−O bonds generate disordered and loosely hydrogen-bonded chains, which enhances the adsorption and activation of toluene. Meanwhile, the dynamic transformation of In−O bond...

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Universal pseudo-fluctuation engineering induces local free radical surface confinement effect to enhance photocatalytic oxidation of toluene

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