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Targeted enhancement of ultra-micropore in highly oxygen-doped carbon derived from biomass for efficient CO2 capture: Insights from experimental and molecular simulation studies

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成果类型:
期刊论文
作者:
Xue, Ruiqi;Xu, Wenjun;Ma, Xiancheng;Guo, Yang;Zeng, Zheng;...
通讯作者:
Xiancheng Ma<&wdkj&>Liqing Li<&wdkj&>Jiayong Si
作者机构:
[Xue, Ruiqi; Xu, Wenjun; Ma, Xiancheng; Si, Jiayong] College of Mechanical and Electrical Engineering, Central South University of Forestry and Technology, Changsha 410004, Hunan, China
[Guo, Yang; Zeng, Zheng; Li, Liqing] School of Energy Science and Engineering, Central South University, Changsha 410083, Hunan, China
通讯机构:
[Xiancheng Ma; Jiayong Si] C
[Liqing Li] S
College of Mechanical and Electrical Engineering, Central South University of Forestry and Technology, Changsha 410004, Hunan, China<&wdkj&>School of Energy Science and Engineering, Central South University, Changsha 410083, Hunan, China
语种:
英文
期刊:
Separation and Purification Technology
ISSN:
1383-5866
年:
2025
卷:
353
页码:
128472
基金类别:
CRediT authorship contribution statement Ruiqi Xue: Writing – original draft, Data curation. Wenjun Xu: Methodology, Investigation. Xiancheng Ma: Writing – review & editing, Investigation, acquisition. Yang Guo: Software, Methodology. Zheng Zeng: Methodology. Liqing Li: Writing – review & editing, Investigation. Jiayong Si: Writing – review & editing, Methodology.
机构署名:
本校为第一且通讯机构
院系归属:
机电工程学院
摘要:
The preparation of efficient CO2 adsorbents is crucial for CO2 capture. Compared to polymer-based carbons and metal-organic frameworks (MOFs), biomass-based carbon exhibits lower adsorption performance. Here, we prepared high oxygen doped ultramicroporous carbon through hydrothermal treatment and mechanical compaction assisted KOH activation. The study found that mechanical compaction treatment can target a 24 % increase in the volume of ultra-micropores, resulting in a CO2 capture of the prepared ultramicroporous carbon reaching 5.6 mmol g−1,...

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