Insights into the synergistic effect of active centers over ZnMg/SBA-15 catalysts in direct synthesis of butadiene from ethanol

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成果类型：

期刊论文

作者：

Wang, Kangzhou;Peng, Xiaobo;Gao, Xinhua;Araki, Yuya;Zhao, Heng;...

通讯作者：

Xiaobo Peng<&wdkj&>Guohui Yang<&wdkj&>Noritatsu Tsubaki

作者机构：

[Xiao, Liwei; Wang, Kangzhou; Araki, Yuya; Liang, Jiaming; Tsubaki, Noritatsu; Zhao, Heng; Yang, Guohui; Peng, Xiaobo] Univ Toyama, Grad Sch Engn, Dept Appl Chem, Gofuku 3190, Toyama 9308555, Japan.

[Gao, Xinhua] Ningxia Univ, Fac Chem & Chem Engn, State Key Lab High Efficiency Utilizat Coal & Gre, Yinchuan 750021, Ningxia, Peoples R China.

[Chen, Jienan] Cent South Univ Forestry & Technol, Minist Forestry, Sch Mat Sci & Engn, Bioethanol Res Ctr, Changsha 410004, Peoples R China.

[Liu, Guangbo; Wu, Jinhu] Chinese Acad Sci, Qingdao Inst Biomass Energy & Bioproc Technol, Qingdao 266101, Peoples R China.

通讯机构：

[Xiaobo Peng; Guohui Yang; Noritatsu Tsubaki] D

Department of Applied Chemistry, Graduate School of Engineering, University of Toyama, Gofuku 3190, Toyama 930-8555, Japan

语种：

英文

期刊：

REACTION CHEMISTRY & ENGINEERING

ISSN：

2058-9883

年：

2021

卷：

期：

页码：

548-558

DOI：

10.1039/d0re00449a

基金类别：

China Scholarship Council (CSC)China Scholarship Council [201807550010]

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

生命科学与技术学院

摘要：

Functionalized catalysts with multiple active centers have been studied in direct conversion of ethanol to butadiene (ETB). However, it is still a considerable challenge to control the synergistic effect of multiple active centers. Here, we report that a series of ZnMg/SBA-15-based catalysts were synthesized for the direct ETB process. The non-polar solvent n-hexane is utilized to improve the synergistic effects of ZnO, MgO and SBA-15. The characterization results demonstrate that the ZnMg/SBA-15-hexane catalyst, prepared from n-hexane solvent, can increase dehydrogenation activity and promote...

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Insights into the synergistic effect of active centers over ZnMg/SBA-15 catalysts in direct synthesis of butadiene from ethanol

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