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In situ growth of Bi/Ag double quantum dots on hollow Bi2MoO6 microspheres: Enhancement of the surface plasmon resonance effect on PMS activation

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成果类型:
期刊论文
作者:
Deng, Yao;Wang, Juntao;Wang, Jing;Zhang, Huidi;Xiao, Hongbo;...
通讯作者:
Wang, WL
作者机构:
[Wang, WL; Xiao, Hongbo; Wang, Wenlei; Deng, Yao] Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Peoples R China.
[Wang, Juntao] Hubei Univ Sci & Technol, Sch Nucl Technol & Chem Biol, Xianning 437100, Peoples R China.
[Wang, Jing; Zhang, Huidi] Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.
[Xiao, Hongbo; Wang, Wenlei; Zhang, Cuihong] Cent South Univ Forestry & Technol, Sch Life Sci & Technol, Changsha 410004, Peoples R China.
通讯机构:
[Wang, WL ] C
Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Peoples R China.
语种:
英文
关键词:
Bi/Ag double quantum dots;Bi2MoO6;SPR effect;PMS activation;CIP degradation
期刊:
Applied Catalysis B: Environmental
ISSN:
0926-3373
年:
2023
卷:
338
页码:
123041
基金类别:
Hunan Huxiang Young Talents Support Program, China [41977129]; National Natural Science Foundation of China [kq1802011]; Changsha Outstanding Innovative Youth Training Program, China [2020JJ4136]; Natural Science Foundation of Hunan Province, China; [2020RC3044]
机构署名:
本校为第一且通讯机构
院系归属:
材料科学与工程学院
生命科学与技术学院
理学院
摘要:
In this work, the effect of Bi/Ag double quantum dots on plasmon resonance and PMS activation was investi-gated. Bi/Ag double quantum dots were generated in situ on hollow Bi2MoO6 microspheres by stepwise irra-diation using a high-energy & beta; electron beam. The formation of Bi/Ag DQDs greatly optimized the drawbacks of Bi2MoO6 in terms of light absorption. Synergistic introduction of DQDs greatly reduced the band gap from 2.72 eV to 2.12 eV. The Bi-Ag@Bi2MoO6 -400/PMS system degraded ciprofloxacin with kinetic constants 10 and 12 times higher than those of the Bi@Bi2MoO6/PMS and Bi2MoO6/PMS...

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