A Promising Strategy for Solvent-Regulated Selective Hydrogenation of 5-Hydroxymethylfurfural over Porous Carbon-Supported Ni-ZnO Nanoparticles

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期刊论文

作者：

Huang, Rulu;Liu, Chao;Zhang, Kaili;Jiang, Jianchun*;Tian, Ziqi;...

通讯作者：

Jiang, Jianchun;Wang, K;Tian, ZQ;Chai, YM

作者机构：

[Jiang, Jianchun; Wang, Kui; Huang, Rulu] Chinese Acad Forestry, Inst Chem Ind Forest Prod, Natl Key Lab Dev & Utilizat Forest Food Resources, Biomass Energy & Mat Key Lab Jiangsu Prov, Nanjing 210042, Peoples R China.

[Jiang, Jianchun; Wang, Kui; Zhang, Kaili; Huang, Rulu] Nanjing Forestry Univ, Coinnovat Ctr Efficient Proc & Utilizat Forest Res, Nanjing 210037, Peoples R China.

[Liu, Chao] Cent South Univ Forestry & Technol, Sch Mat Sci & Engn, Changsha 410004, Peoples R China.

[Tian, Ziqi] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China.

[Chai, Yongming] China Univ Petr East China, Coll Chem & Chem Engn, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China.

通讯机构：

[Chai, YM ; Wang, K ; Jiang, JC; Tian, ZQ ] C

Chinese Acad Forestry, Inst Chem Ind Forest Prod, Natl Key Lab Dev & Utilizat Forest Food Resources, Biomass Energy & Mat Key Lab Jiangsu Prov, Nanjing 210042, Peoples R China.

Nanjing Forestry Univ, Coinnovat Ctr Efficient Proc & Utilizat Forest Res, Nanjing 210037, Peoples R China.

Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China.

China Univ Petr East China, Coll Chem & Chem Engn, State Key Lab Heavy Oil Proc, Qingdao 266580, Peoples R China.

语种：

英文

关键词：

Porous carbon-supported Ni-ZnO nanoparticles catalyst;Selective hydrogenation;5-Hydroxymethylfurfural;Solvent;Proton-donating ability

期刊：

纳微快报(英文)

ISSN：

2311-6706

年：

2026

卷：

期：

页码：

1-14

DOI：

10.1007/s40820-025-01847-5

基金类别：

National Nature Science Foundation of China for Excellent Young Scientists Fund [32222058]; Fundamental Research Foundation of CAF [CAFYBB2022QB001]

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

Developing biomass platform compounds into high value-added chemicals is a key step in renewable resource utilization. Herein, we report porous carbon-supported Ni-ZnO nanoparticles catalyst (Ni-ZnO/AC) synthesized via low-temperature coprecipitation, exhibiting excellent performance for the selective hydrogenation of 5-hydroxymethylfurfural (HMF). A linear correlation is first observed between solvent polarity (ET(30)) and product selectivity within both polar aprotic and protic solvent classes, suggesting that solvent properties play a vital role in directing reaction pathways. Among these, ...

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A Promising Strategy for Solvent-Regulated Selective Hydrogenation of 5-Hydroxymethylfurfural over Porous Carbon-Supported Ni-ZnO Nanoparticles

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