Direct carbonyl reductive functionalizations by diphenylphosphine oxide

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期刊论文

作者：

Liu, Feng;Dong, Jianyu;Cheng, Ruofei;Yin, Shuang-Feng;Chen, Lang;...

通讯作者：

Zhou, YB;Dong, JY;Li, CJ

作者机构：

[Zhou, Yongbo; Yin, Shuang-Feng; Qiu, Renhua; Han, Li-Biao; Zhou, YB; Chen, Lang; Liu, Feng; Su, Lebin] Hunan Univ, Coll Chem & Chem Engn, Adv Catalyt Engn Res Ctr, Minist Educ, Changsha 410082, Peoples R China.

[Dong, JY; Dong, Jianyu] Hunan First Normal Univ, Sch Phys & Chem, Changsha 410205, Peoples R China.

[Li, Chao-Jun; Cheng, Ruofei] McGill Univ, FQRNT Ctr Green Chem & Catalysis, Dept Chem, 801 Sherbrooke St W, Montreal, PQ H3A 0B8, Canada.

[Yin, Shuang-Feng] Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Peoples R China.

通讯机构：

[Zhou, YB ; Dong, JY ] H

[Li, CJ ] M

Hunan Univ, Coll Chem & Chem Engn, Adv Catalyt Engn Res Ctr, Minist Educ, Changsha 410082, Peoples R China.

Hunan First Normal Univ, Sch Phys & Chem, Changsha 410205, Peoples R China.

McGill Univ, FQRNT Ctr Green Chem & Catalysis, Dept Chem, 801 Sherbrooke St W, Montreal, PQ H3A 0B8, Canada.

语种：

英文

期刊：

Science Advances

ISSN：

2375-2548

年：

2025

卷：

期：

页码：

eads4626

DOI：

10.1126/sciadv.ads4626

基金类别：

National Natural Science Foundation of China : 22471065, 21878072, 21573065 National Natural Science Foundation of China : 22471065, 21706058 National Natural Science Foundation of China : 21938002 National Key Research and Development Program: 2022YFB4002400 Hunan Provincial Natural Science Foundation of China: 2020JJ2011 Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang: 2022R01021 The Canada Research Chair Foundation The FQRNT Center for Green Chemistry and Catalysis The National Science and Engineering Research Center The Centre in Green Chemistry and Catalysis

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本校为其他机构

院系归属：

理学院

摘要：

Reductive functionalization of aldehydes and ketones is one of the most challenging but ultimately rewarding areas in synthetic chemistry and related sciences. We report a simple and extremely versatile carbonyl reductive functionalization strategy achieving direct, highly selective, and efficient reductive amination, etherification, esterification, and phosphinylation reactions of (hetero)aryl aldehydes and ketones, which are extremely challenging or unattainable to achieve by traditional strategies, using only diphenylphosphine oxide and an inorganic base. It enables modular synthesis of fun...

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Direct carbonyl reductive functionalizations by diphenylphosphine oxide

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