Mesoporous TiO2 Mesocrystals: Remarkable Defects-Induced Crystallite-Interface Reactivity and Their in Situ Conversion to Single Crystals

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成果类型：

期刊论文

作者：

Liu, Yong;Luo, Yongfeng;Elzatahry, Ahmed A.;Luo, Wei;Che, Renchao;...

通讯作者：

Zhao, Dongyuan

作者机构：

[Yao, Chi; Che, Renchao; Tang, Yun; Wang, Chun; Zhao, Dongyuan; Sun, Zhenkun; Shen, Dengke; Gao, Wenjun; Deng, Yonghui; Zhou, Gang; Ling, Yun; Lan, Kun; Li, Bin; Luo, Wei; Yuan, Kaiping; Luo, Yongfeng; Liu, Yong; Wang, Jingxiu; Zheng, Gengfeng; Fan, Jianwei; Liu, Zhengwang] Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Dept Chem, State Key Lab Mol Engn Polymers,Lab Adv Mat, Shanghai 200433, Peoples R China.

[Luo, Yongfeng] Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Hunan, Peoples R China.

[Elzatahry, Ahmed A.] Qatar Univ, Coll Arts & Sci, Mat Sci & Technol Program, Doha, Qatar.

[Luo, Wei] Donghua Univ, Coll Mat Sci & Engn, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China.

[Fan, Jianwei] Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 200092, Peoples R China.

通讯机构：

[Zhao, Dongyuan] F

Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Dept Chem, State Key Lab Mol Engn Polymers,Lab Adv Mat, Shanghai 200433, Peoples R China.

语种：

英文

期刊：

ACS CENTRAL SCIENCE

ISSN：

2374-7943

年：

2015

卷：

期：

页码：

400-408

DOI：

10.1021/acscentsci.5b00256

基金类别：

This work is supported by the State Key Basic Research Program of China (2013CB934104 and 2012CB224805), the National Science Foundation (21210004) and Science & Technology Commission of Shanghai Municipality (14JC1400700), Shanghai Leading Academic Discipline Project (B108), and Deanship of Scientific Research, KSU-The International Highly Cited Research Group program (IHCRG#14-102). Y.L. also acknowledges the Interdisciplinary Outstanding Doctoral Research Funding of Fudan University (EZH2203302/001).

机构署名：

本校为其他机构

院系归属：

理学院

摘要：

Oriented self-assembly between inorganic nanocrystals and surfactants is emerging as a route for obtaining new mesocrystalline semiconductors. However, the actual synthesis of mesoporous semiconductor mesocrystals with abundant surface sites is extremely difficult, and the corresponding new physical and chemical properties arising from such an intrinsic porous mesocrystalline nature, which is of fundamental importance for designing high-efficiency nanostructured devices, have been rarely explored and poorly understood. Herein, we report a simpl...

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Mesoporous TiO2 Mesocrystals: Remarkable Defects-Induced Crystallite-Interface Reactivity and Their in Situ Conversion to Single Crystals

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