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In situ regulation of the oxygen vacancy concentration of Bi4Ti3O12 by β-particles to activate peroxydisulfate

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成果类型:
期刊论文
作者:
Tan, Binbin;Wang, Jing;Deng, Yao;Zhang, Huidi;Wang, Jiang;...
通讯作者:
Wang, WL
作者机构:
[Wang, WL; Wang, Wenlei; Tan, Binbin; Deng, Yao; Wang, Jiang] Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Peoples R China.
[Wang, Jing; Zhang, Huidi; Zhang, Zhihao] Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.
[Wang, Wenlei] Cent South Univ Forestry & Technol, Inst Chem Disposal & Resource Utilizat Hazardous W, Changsha 410004, Peoples R China.
通讯机构:
[Wang, WL ] C
Cent South Univ Forestry & Technol, Coll Sci, Changsha 410004, Peoples R China.
语种:
英文
关键词:
Oxygen vacancies;In-situ regulation;Peroxydisulfate;CIP degradation
期刊:
Applied Surface Science
ISSN:
0169-4332
年:
2024
卷:
649
页码:
159134
基金类别:
Hunan Huxiang Young Talents Support Program, China [2020RC3044]; Natural Science Foundation of Hunan Province, China [2020JJ4136]; National Natural Science Foundation of China [41977129]; Changsha Outstanding Innovative Youth Training Program, China [kq1802011]
机构署名:
本校为第一且通讯机构
院系归属:
材料科学与工程学院
理学院
摘要:
The key to enhancing the activation efficiency of peroxydisulfate (PDS) lies in facilitating the adsorption of PDS and accelerating the rate of electron transfer at the interface. In this work, the oxygen vacancy (Ovs) concentration of ultrathin Bi4Ti3O12 (BTO) was controlled in situ by high-energy electron beam bombardment. BTOV- 300 exhibited a significant activation effect on PDS. The degradation rate constant (kobs) for the removal of ciprofloxacin (CIP) was measured to be 0.2080 min  1 under visible light irradiation, which was 3.71 time...

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