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Construction of g-C3N4 with N2C-type defects/MoO3 Z-scheme photocatalyst: Effective mineralization and toxicity reduction of microcystin-LR by multiple free radical degradation pathways

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成果类型:
期刊论文
作者:
Ouyang, Yuanhao;Jiang, Honghui;Zhong, Haoxiang;Li, Guoyu;Ji, Xiaodong;...
通讯作者:
Hu, Xinjiang(xjhu@csuft.edu.cn)
作者机构:
[Jiang, Honghui; Ouyang, Yuanhao; Hu, Xinjiang; Li, Guoyu; Xue, Wei; Zhong, Haoxiang; Ji, Xiaodong] Cent South Univ Forestry & Technol, Coll Environm Sci & Engn, Changsha 410004, Peoples R China.
[Jin, Qi] Univ Sci & Technol Beijing, Sch Energy & Environm Engn, Beijing 100083, Peoples R China.
[Zhu, Mingshan] Jinan Univ, Sch Environm, Guangdong Key Lab Environm Pollut & Hlth, Guangzhou, Peoples R China.
通讯机构:
[Xinjiang Hu] C
[Mingshan Zhu] G
College of Environmental Science and Engineering, Central South University of Forestry and Technology, Changsha 410004, PR China<&wdkj&>Guangdong Key Laboratory of Environmental Pollution and Health, School of Environment, Jinan University, Guangzhou 511443, PR China
语种:
英文
关键词:
Microcystis-LR;Degradation
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2023
卷:
464
页码:
142542
基金类别:
National Natural Science Foundation of China [51979294]; Training Program for Excellent Young Innovators of Changsha [kq1905064]
机构署名:
本校为第一机构
院系归属:
环境科学与工程学院
摘要:
Algal blooms have resulted in the buildup of microcystin (MC-LR) in water bodies, posing a severe hazard to the safety of the aquatic ecosystem and human health. This study produced a g-C3N4 with N2C-type defects/MoO3 Z-scheme photocatalyst (D-CN/MoO3) for MC-LR degradation in visible light. D-CN/MoO3 could photodegrade 100 % MC-LR within 25 min, which was substantially more significant than pure g-C3N4 (12.5%). Meanwhile, the kinetic constant was 32.5 times higher than pure g-C3N4, attributed to the defect engineering and Z-scheme heterojuncti...

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