Green and rapid synthesis of hierarchical nano-sized pure Si-Beta zeolite supported with Zn and Y for effective synthesis of butadiene from aqueous ethanol

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成果类型：

期刊论文

作者：

Wang, Kangzhou;Chen, Chong;Gao, Weizhe*;Liu, Na;Wang, Chengwei;...

通讯作者：

Gao, Weizhe;Tsubaki, N

作者机构：

[Chen, Chong; Wang, Kangzhou] Ningxia Univ, Sch Mat & New Energy, Yinchuan 750021, Ningxia, Peoples R China.

[Wang, Chengwei; Fan, Jiaqi; Tsubaki, Noritatsu; Tsubaki, N; Gao, Weizhe; Gu, Yongqiang; Zhu, Caixia; Wang, Fan; Gao, WZ] Univ Toyama, Sch Engn, Dept Appl Chem, Gofuku 3190, Toyama 9308555, Japan.

[Liu, Na] Cent South Univ Forestry & Technol, Sch Mat Sci & Engn, Changsha 410004, Hunan, Peoples R China.

通讯机构：

[Tsubaki, N ; Gao, WZ] U

Univ Toyama, Sch Engn, Dept Appl Chem, Gofuku 3190, Toyama 9308555, Japan.

语种：

英文

关键词：

Aqueous ethanol;Butadiene;pure Si-Beta;Hierarchical nano-sized structure;Acid-base properties

期刊：

Chemical Engineering Journal

ISSN：

1385-8947

年：

2024

卷：

479

页码：

147780

DOI：

10.1016/j.cej.2023.147780

基金类别：

Innovation and Entrepreneurship Training Program for College Students of Ningxia University, China

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

Direct synthesis of butadiene (BD) from aqueous ethanol is a promising route, but the development of novel supports and the yield of BD still confronts significant challenges. Herein, we report the green and rapid synthesis method of hierarchical nano-sized pure Si-Beta zeolite, which drastically reduces the crystallization time and avoids the use of HF as well as the generation of large amounts of wastewater compared to the conventional pure Si-Beta zeolite synthesis. Meanwhile, the synthesized hierarchical nano-sized pure Si-Beta zeolite supported with Zn and Y achieved more than 60 % for BD...

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Green and rapid synthesis of hierarchical nano-sized pure Si-Beta zeolite supported with Zn and Y for effective synthesis of butadiene from aqueous ethanol

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