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Large Seasonal Variation in Nitrogen Isotopic Abundances of Ammonia Volatilized from a Cropland Ecosystem and Implications for Regional NH3 Source Partitioning

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成果类型:
期刊论文
作者:
Song, Linlin;Wang, Ang;Li, Zhengjie;Kang, Ronghua;Walters, Wendell W.;...
通讯作者:
Fang, YT
作者机构:
[Kang, Ronghua; Quan, Zhi; Song, Linlin; Fang, Yunting; Wang, Ang] Chinese Acad Sci, CAS Key Lab Forest Ecol & Management, Inst Appl Ecol, Shenyang 110016, Liaoning, Peoples R China.
[Kang, Ronghua; Quan, Zhi; Song, Linlin; Fang, Yunting; Wang, Ang] Key Lab Stable Isotope Tech & Applicat, Shenyang 110016, Liaoning, Peoples R China.
[Li, Zhengjie] Cent South Univ Forestry & Technol, Coll Biol Sci & Technol, Changsha 410004, Hunan, Peoples R China.
[Walters, Wendell W.] Univ South Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA.
[Pan, Yuepeng] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atmo, Beijing 100029, Peoples R China.
通讯机构:
[Fang, YT ] C
Chinese Acad Sci, CAS Key Lab Forest Ecol & Management, Inst Appl Ecol, Shenyang 110016, Liaoning, Peoples R China.
Key Lab Stable Isotope Tech & Applicat, Shenyang 110016, Liaoning, Peoples R China.
Chinese Acad Sci, Qingyuan Forest CERN, Shenyang 110016, Liaoning, Peoples R China.
语种:
英文
关键词:
dynamic variation;isotopic fractionation;nitrogen isotopic signatures;northeast China;soil ammonia emissions;source apportionment
期刊:
Environmental Science & Technology
ISSN:
0013-936X
年:
2024
卷:
58
期:
2
页码:
1177-1186
基金类别:
Hundred Talents Program of Chinese Academy of Sciences [XDA28020302]; Strategic Priority Research Program of the Chinese Academy of Sciences [2017YFC0212700]; National Key R&D Program of China [DQGG0105-02]; National Research Program for Key Issues in Air Pollution Control [32271671, 42077204]; National Natural Science Foundation of China [2022194]; Youth Innovation Promotion Association CAS [2019000186]; Hundred Talents Program of Chinese Academy of Sciences [2021JJ41071]; Natural Science Foundation of Hunan Province [XLYC1902016]; Liaoning Vitalization Talents Program
机构署名:
本校为其他机构
摘要:
Ammonia (NH3) volatilization from agricultural lands is a main source of atmospheric reduced nitrogen species (NHx). Accurately quantifying its contribution to regional atmospheric NHx deposition is critical for controlling regional air nitrogen pollution. The stable nitrogen isotope composition (expressed by delta N-15) is a promising indicator to trace atmospheric NHx sources, presupposing a reliable nitrogen isotopic signature of NH3 emission sources. To obtain more specific seasonal delta N-15 values of soil NH3 volatilization for reliable regional seasonal NH3 source partitioning, we util...

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