Sublayer-Sulfur-Vacancy-Induced Charge Redistribution of FeCuS Nanoflower Awakening Alkaline Hydrogen Evolution

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期刊论文

作者：

Liu, Li;Xu, Jie;Cao, Jinming;Liu, Yangxi;Bai, Yuanjuan;...

通讯作者：

Liu, L;Ma, XG;Yang, XH

作者机构：

[Liu, Li; Xu, Jie; Liu, L; Cao, Jinming; Liu, Yangxi] Chongqing Normal Univ, Coll Chem, Chongqing Key Lab Green Catalysis Mat & Technol, Chongqing 401331, Peoples R China.

[Bai, Yuanjuan] Cent South Univ Forestry & Technol, Coll Mat Sci & Engn, Changsha 410004, Peoples R China.

[Ma, Xinguo] Hubei Univ Technol, Sch Sci, Wuhan 430068, Hubei, Peoples R China.

[Yang, XH; Yang, Xiaohui] Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China.

通讯机构：

[Yang, XH ; Liu, L ] C

[Ma, XG ] H

Chongqing Normal Univ, Coll Chem, Chongqing Key Lab Green Catalysis Mat & Technol, Chongqing 401331, Peoples R China.

Hubei Univ Technol, Sch Sci, Wuhan 430068, Hubei, Peoples R China.

Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China.

语种：

英文

期刊：

INORGANIC CHEMISTRY

ISSN：

0020-1669

年：

2024

DOI：

10.1021/acs.inorgchem.4c00915

基金类别：

Chongqing Normal University [KJZD-M202200503]; Science and Technology Research Program of Chongqing Municipal Education Commission [CSTB2022NSCQ-LZX0077]; Natural Science Foundation Joint Fund for Innovation and Development of Chongqing Municipal Education Commission [52100065]; National Natural Science Foundation of China [CXQT21015]; Chongqing Innovation Research Group Project [02060404/2020009000321]; Doctor Start/Talent Introduction Program of Chongqing Normal University

机构署名：

本校为其他机构

院系归属：

材料科学与工程学院

摘要：

Advancing the progress of sustainable and green energy technologies requires the improvement of valid electrocatalysts for the hydrogen evolution reaction (HER). Reconfiguring charge distribution through heteroatom doping-induced vacancy serves as an effective approach to implement high performance for HER catalysts. Here, we successfully fabricated Fe-doped CuS (FeCuS) with the sublayer sulfur vacancy to judge its HER performance and dissect the activity origins. Density functional theory calculation further elucidates that the primary factor contributing to the heightened HER activity is tha...

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Sublayer-Sulfur-Vacancy-Induced Charge Redistribution of FeCuS Nanoflower Awakening Alkaline Hydrogen Evolution

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