Green and sustainable alternatives to petroleum-based plastics can reduce  environmental pollution and alleviate the resource crisis. Reed straw (Rs) is a  rapidly growing, eco-friendly, low-cost, and natural fiber with great potential  as a sustainable resource. However, the development of high-performance plastic  substitutes from Rs is challenging owing to its weak interfacial bonding. Herein,  inspired by the structure of reinforced concrete, a top-down strategy is adopted  using a simple and rapid physical-filling and directional-assembly method...