Tungsten carbide induced acceleration of Fe3+/Fe2+cycle in Fe2+/PMS process for rapid degradation of tetracycline hydrochloride

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期刊论文

作者：

Cheng, Hao;Liu, Hao;Huang, Chao*;Xu, Jialu;Tian, Haoran;...

通讯作者：

Huang, Chao;Wang, P

作者机构：

[Wang, Ping; Cheng, Hao; Huang, Chao; Yang, Jikun; Tian, Haoran; Xu, Jialu; Cai, Jingju] Cent South Univ Forestry & Technol, Coll Environm Sci & Engn, Changsha 410004, Peoples R China.

[Liu, Hao] China Machinery Int Engn Design & Res Inst Co Ltd, Changsha 410000, Peoples R China.

[Cheng, Min] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Peoples R China.

[Liu, Zhiming] Eastern New Mexico Univ, Dept Biol, Portales, NM 88130 USA.

通讯机构：

[Wang, P ; Huang, C] C

Cent South Univ Forestry & Technol, Coll Environm Sci & Engn, Changsha 410004, Peoples R China.

语种：

英文

关键词：

Tungsten carbide (WC);Peroxymonosulfate (PMS);Co-catalytic;Fenton-like process;Tetracycline hydrochloride (TC)

期刊：

Separation and Purification Technology

ISSN：

1383-5866

年：

2024

卷：

330

DOI：

10.1016/j.seppur.2023.125311

基金类别：

National Natural Science Foundation of China [51809293, 22102219]; Natural Science Foundation of Hunan Province [2023JJ31007]; Scientific Research Staring Foundation for the Attracted Talent of Central South University of Forestry and Technology [2018YJ016]

机构署名：

本校为第一且通讯机构

院系归属：

环境科学与工程学院

摘要：

Metal sulfides have gained significant attention as cocatalysts for Fenton/Fenton-like processes in recent years due to their ability to reduce trivalent iron (Fe3+). Nevertheless, the issue of hydrogen sulfide (H2S) formation as a secondary contaminant is a significant concern. In this work, tungsten carbide (WC) was innovatively intro-duced into the Fenton-like process based on ferrous ion/peroxymonosulfate (Fe2+/PMS). The results showed that the WC/Fe2+/PMS system had a significantly higher degradation efficiency and rate for tetracycline hydro-chloride (TC) than the Fe2+/PMS system. The WC...

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Tungsten carbide induced acceleration of Fe3+/Fe2+cycle in Fe2+/PMS process for rapid degradation of tetracycline hydrochloride

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