Accurately mapping forest carbon density by combining sample plots and remotely sensed images has become popular because this method provides spatially explicit estimates. However, mixed pixels often impede the improvement of the estimation. In this letter, regression modeling and spectral unmixing analysis were integrated to improve the estimation of forest carbon density for the You County of Hunan, China, using Landsat Thematic Mapper images. Linear spectral unmixing with and without a constraint (LSUWC and LSUWOC) and nonlinear spectral unm...