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Adsorption of estrogen contaminants (17β-estradiol and 17α-ethynylestradiol) by graphene nanosheets from water: Effects of graphene characteristics and solution chemistry

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成果类型:
期刊论文
作者:
Jiang, Luhua;Liu, Yunguo*;Zeng, Guangming;Liu, Shaobo;Hu, Xinjiang;...
通讯作者:
Liu, Yunguo
作者机构:
[Jiang, Luhua; Liu, Yunguo; Zeng, Guangming; Tan, Xiaofei; Li, Meifang; Liu, Ni] Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
[Jiang, Luhua; Liu, Yunguo; Zeng, Guangming; Tan, Xiaofei; Li, Meifang; Liu, Ni] Hunan Univ, Minist Educ, Key Lab Environm Biol & Pollut Control, Changsha 410082, Hunan, Peoples R China.
[Liu, Shaobo] Cent S Univ, Sch Met & Environm, Changsha 410083, Peoples R China.
[Hu, Xinjiang] Cent South Univ Forestry & Technol, Coll Environm Sci & Engn Res, Changsha 410004, Hunan, Peoples R China.
[Zhou, Lu] Changsha Univ Sci & Technol, Sch Hydraul Engn, Changsha 410004, Hunan, Peoples R China.
通讯机构:
[Liu, Yunguo] H
Hunan Univ, Coll Environm Sci & Engn, Changsha 410082, Hunan, Peoples R China.
语种:
英文
关键词:
Estrogen contaminants;Graphene nanosheets;Natural organic matter;Reduction degree
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2018
卷:
339
页码:
296-302
基金类别:
This subject has been supported by the National Natural Science Foundation of China (Grants No. 51521006 , 51609268 and 51608208 ), the Hunan Provincial Innovation Foundation for Postgraduate (Grant No. CX2016B135 ), and the Key Project of Technological Innovation in the Field of Social Development of Hunan Province, China (Grant Nos. 2016SK2010 and 2016SK2001 ).
机构署名:
本校为其他机构
院系归属:
环境科学与工程学院
摘要:
In this research, adsorption of two estrogens, namely, 17β-estradiol (E2) and 17α-ethynylestradiol (EE2), by graphene nanosheets with different reduction degrees (rGOs) were investigated;and the effects of solution chemistry, such as natural organic matter (NOM), pH and ionic strength (IS), on the E2 and EE2 adsorption behaviors were also examined. Results indicated that adsorption abilities of estrogens increased with increasing the reduction degree of rGOs;the π–πstacking interaction could be considered as a predominant interaction to the enhanced adsorption capacities...

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